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Oxide Molecular Beam Epitaxy Group
Group Members
Gennady Logvenov
Member of MBE Group
from 2004 to 2009
Current Position
Senior Scientist and Group Leader
Max Planck Institute for Solid State Research
Publications in high-impact journals while in the MBE GroupJ. Wu, O. Pelleg, G. Logvenov, A. T. Bollinger, Y. Sun, G. S. Boebinger, M. Vanevic, Z. Radovic and I. Bozovic. “Anomalous (in)dependence of interface superconductivity on carrier density.” Nature Materials (Submitted 2012). In press. | X. Shi, G. Logvenov, A. T. Bollinger, I. Bozovic, C. Panagopoulos and D. Popovic. “Emergence of superconductivity from the dynamically heterogeneous insulating state in La2-xSrxCuO4” Nature Materials 12, 47-51 (2013). | L. S. Bilbro, R. V. Aguilar, G. Logvenov, O. Pelleg, I. Bozovic and N. P. Armitage. “Temporal correlations of superconductivity above the transition temperature in La2-xSrxCuO4 probed by terahertz spectroscopy.” Nature Physics 7, 298-302 (2011). | E. Morenzoni, B. M. Wojek, A. Suter, T. Prokscha, G. Logvenov and I. Bozovic. “The Meissner effect in a strongly underdoped cuprate above its critical temperature.” Nature Communications 2, 272 (2011). | H. Zhou, Y. Yacoby, V. Y. Butko, G. Logvenov, I. Bozovic and R. Pindak. “Anomalous expansion of the copper-apical-oxygen distance in superconducting cuprate bilayers.” Proceedings of the National Academy of Sciences 107, 8103-8107 (2010). | A. Suter, E. Morenzoni, T. Prokscha, B. M. Wojek, H. Luetkens, G. Nieuwenhuys, A. Gozar, G. Logvenov and I. Bozovic. “Two-Dimensional Magnetic and Superconducting Phases in Metal-Insulator La2-xSrxCuO4 Superlattices Measured by Muon-Spin Rotation.” Physical Review Letters 106 (2011). | I. Sochnikov, A. Shaulov, Y. Yeshurun, G. Logvenov and I. Bozovic. “Large oscillations of the magnetoresistance in nanopatterned high-temperature superconducting films.” Nature Nanotechnology 5, 516-519 (2010). | G. Logvenov, A. Gozar and I. Bozovic. “High-Temperature Superconductivity in a Single Copper-Oxygen Plane.” Science 326, 699 (2009). Abstract
The question of how thin cuprate layers can be while still retaining high-temperature
superconductivity (HTS) has been challenging to address, in part because experimental studies
require the synthesis of near-perfect ultrathin HTS layers and ways to profile the superconducting
properties such as the critical temperature and the superfluid density across interfaces with atomic
resolution. We used atomic-layer molecular beam epitaxy to synthesize bilayers of a cuprate metal
(La1.65Sr0.45CuO4) and a cuprate insulator (La2CuO4) in which each layer is just three unit cells
thick. We selectively doped layers with isovalent Zn atoms, which suppress superconductivity and
act as markers, to show that this interface HTS occurs within a single CuO2 plane. This approach
may also be useful in fabricating HTS devices. | V. Y. Butko, G. Logvenov, N. Bozovic, Z. Radovic and I. Bozovic. “Madelung Strain in Cuprate Superconductors - A Route to Enhancement of the Critical Temperature.” Advanced Materials 21, 3644 (2009). Abstract
"Madelung Strain" in cuprate films containing metal (M = La1.56Sr0.44CuO4)
and insulator (I = La2CuO4) layers: X-ray diffraction shows that, unexpectedly, the volume
of unit cell of the top layer adjusts to that of the bottom layer. The effect is due to
long-range Coulomb forces; it affects interfacial superconductivity because the critical
temperature scales with the unit-cell height. | S. Smadici, J. C. T. Lee, S. Wang, P. Abbamonte, G. Logvenov, A. Gozar, C. D. Cavellin and I. Bozovic. “Superconducting Transition at 38 K in Insulating-Overdoped La2CuO4-La1.64Sr0.36CuO4 Superlattices: Evidence for Interface Electronic Redistribution from Resonant Soft X-Ray Scattering.” Physical Review Letters 102, 107004 (2009). Abstract
We use resonant soft x-ray scattering (RSXS) to quantify the hole distribution in a superlattice of
insulating La2CuO4 (LCO) and overdoped La2-xSrxCuO4 (LSCO). Despite its nonsuperconducting constituents,
this structure is superconducting with Tc=38 K. We found that the conducting holes redistribute
electronically from LSCO to the LCO layers. The LCO layers were found to be optimally doped, suggesting
they are the main drivers of superconductivity. Our results demonstrate the utility of RSXS for
separating electronic from structural effects at oxide interfaces. | H. Shim, P. Chaudhari, G. Logvenov and I. Bozovic. “Electron-Phonon Interactions in Superconducting La1.84Sr0.16CuO4 Films.” Physical Review Letters 101, 247004 (2008). Abstract
We have measured quasiparticle tunneling across a junction perpendicular to the superconducting
copper oxide planes. The tunneling spectra show peaks in the density of states. There are 11 minima
in the second derivative d(2)I/dV(2), where I is the current and V the voltage, suggesting multiple
boson-quasiparticle interactions. These minima match precisely with the published Raman scattering
data, leading us to conclude that the relevant bosons in superconducting La1.84Sr0.16CuO4 films are
phonons. | A. Gozar, G. Logvenov, L. F. Kourkoutis, A. T. Bollinger, L. A. Giannuzzi, D. A. Muller and I. Bozovic. “High-temperature interface superconductivity between metallic and insulating copper oxides.” Nature 455, 782 (2008). Abstract
The realization of high- transition- temperature (high-Tc) superconductivity confined
to nanometre-sized interfaces has been a long- standing goal because of potential
applications(1,2) and the opportunity to study quantum phenomena in reduced dimensions(3,4).
This has been, however, a challenging target: in conventional metals, the high electron
density restricts interface effects (such as carrier depletion or accumulation) to a
region much narrower than the coherence length, which is the scale necessary for superconductivity
to occur. By contrast, in copper oxides the carrier density is low whereas Tc is high and the
coherence length very short, which provides an opportunity - but at a price: the interface must
be atomically perfect. Here we report superconductivity in bilayers consisting of an insulator
(La2CuO4) and a metal (La1.55Sr0.45CuO4), neither of which is superconducting in isolation.
In these bilayers, Tc is either similar to 15 K or similar to 30 K, depending on the layering
sequence. This highly robust phenomenon is confined within 2 - 3nm of the interface. If such a
bilayer is exposed to ozone, Tc exceeds 50 K, and this enhanced superconductivity is also shown
to originate from an interface layer about 1 - 2 unit cells thick. Enhancement of Tc in bilayer
systems was observed previously(5) but the essential role of the interface was not recognized at
the time. | N. Gedik, D. S. Yang, G. Logvenov, I. Bozovic and A. H. Zewail. “Nonequilibrium phase transitions in cuprates observed by ultrafast electron crystallography.” Science 316, 425 (2007). Abstract
Nonequilibrium phase transitions, which are defined by the formation of macroscopic transient
domains, are optically dark and cannot be observed through conventional temperature- or pressure-change
studies. We have directly determined the structural dynamics of such a nonequilibrium phase transition
in a cuprate superconductor. Ultrafast electron crystallography with the use of a tilted optical geometry
technique afforded the necessary atomic-scale spatial and temporal resolutions. The observed transient behavior
displays a notable "structural isosbestic" point and a threshold effect for the dependence of
c-axis expansion (Delta c) on fluence (F), with Delta c/F = 0.02 angstrom/(millijoule per square
centimeter). This threshold for photon doping occurs at similar to 0.12 photons per copper site,
which is unexpectedly close to the density (per site) of chemically doped carriers needed to induce
superconductivity. | I. Bozovic, G. Logvenov, M. A. J. Verhoeven, P. Caputo, E. Goldobin and M. R. Beasley. “Giant proximity effect in cuprate superconductors.” Physical Review Letters 93, 157002 (2004). Abstract
Using an advanced molecular beam epitaxy system, we have reproducibly synthesized atomically smooth films of high-temperature superconductors and uniform trilayer junctions with virtually perfect interfaces. We found that supercurrent runs through very thick barriers. We can rule out pinholes and microshorts; this "giant proximity effect" (GPE) is intrinsic. It defies the conventional explanation; it might originate in resonant tunneling through pair states in an almost-superconducting barrier. GPE may also be significant for superconducting electronics, since thick barriers are easier to fabricate. |
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