Tracer Technology Group

Local Projects

PFTs have been widely used to provide data for model verification and refinement on the scale of a few to tens of miles.  Two major experiments in which BNL applied PFT tracer technology are the Vertical transport and mixing (VTMX) experiment held in Salt Lake City in 2000 and the Urban Dispersion Program being conducted from 2004 - 2007. 

A meteorological field measurement program was conducted in the Salt Lake Valley during October 2000. Scientists from government laboratories, universities, and private industry carried out studies of the processes contributing to the vertical transport and mixing of momentum, heat, and water vapor in the lowest few thousand feet of the atmosphere. Such processes affect how wind speed, temperature, and moisture vary with height and how atmospheric pollutants may be distributed over an area. Vertical transport and mixing (VTMX) processes play a significant but not yet well-defined role in the transport, dilution, and subsequent fate of pollutants in urban basins located within intermountain basin regions.  In the VTMX program, the important role of tracers in following the effects of these processes has been recognized and the perfluorocarbon tracer (PFT) technology was used in this four-year program (more...).  The results of this work program increased the fundamental understanding of these phenomena, which may eventually lead to improved air quality and weather forecasting models (more...).

The New York City Urban Dispersion Program is a four-year (2004-2007) multi-National Laboratory, multi-Federal Agency research project whose major objective is to study how air flows in a city environment. The deep canyons created by the tall buildings in New York create challenges in predicting air flow. Field studies using perfluorocarbon gas tracers have been and will be performed to provide data that can help improve and validate computer models that simulate the atmospheric movement of contaminants within cities, and around, into and building interiors and subways (more...).

Ameriflux Tower Footprint Studies

 There is a natural cycle in which CO2 moves between the atmosphere and the ocean and the atmosphere and the terrestrial biosphere.  Understanding the dynamics of the carbon cycle is essential to predicting future atmospheric CO2 levels.  Eddy covariance methods are used at AmeriFlux sites to measure the net ecosystem exchange (NEE) as measured by the flux of CO2, H2O and other fluxes.  These techniques have limitations.  Generalization of tower flux results requires a detailed knowledge of the degree to which the area responsible for the flux of CO2 and other gases at the measurement site (the footprint) represents the regional biosphere.  There are also other problems with eddy correlation methods that occur during periods of strong atmospheric stability, particularly during calm nocturnal periods.  PFT Studies are being conducted in Florida and the Savannah River Site to resolve some of these issues.

Florida

The Florida Footprint experiments were a series of field programs in which perfluorocarbon tracers were released in different configurations centered around a flux tower.  The concentrations of these tracers were measured at different levels on the tower.  These data will be compared to the meteorological and CO2 flux data to determine relationships between the tower footprint, the measured fluxes and the meteorological conditions and will be used to improve and validate models used to predict tower footprints.  Details can be found at (more...)

Savannah River Super Site Studies

There have been a limited number of experiments designed to validate footprint models, and address the applicability of applying current models and the problems with using them in non-ideal conditions.  Previous tracer experiments to validate footprint models have been conducted using a single tracer, SF6 and have not been preformed under stable nocturnal conditions. 

The nocturnal boundary layer technique (NBL) has been presented as a possible alternative to the eddy covariance technique for the determination of CO2 and other fluxes in stable nighttime conditions.  This technique is based on the assumption that the nocturnal boundary layer is isolated from the upper levels of the atmosphere and the effects of surface sources and sinks are trapped in this relatively shallow layer.

In the summer of 2007 we will conduct a series of annual Perfluorocarbon Tracer (PFT) experiments at the Integrated Carbon Flux Super-site.  These programs are funded by the Department of Energy Terrestrial Carbon program.  The goals of the PFT experiments will be to test the NBL method under a variety of meteorological conditions, determine the effects of the Low Level Jet (LLJ) on surface fluxes and their measurement, map the tower flux footprint under different atmospheric conditions and examine the effects on CO2 measurements at the tower, and quantify the effects of inhomogenities in the flux source region, and examine effects of non-local forcing on fluxes at the tower. 

The tracer concentration data will be used to empirically determine the tower footprint.  The data will be compared with models prediction of footprints.  These data will be compared to the meteorological and CO2 flux data to determine relationships between the tower footprint, the measured fluxes and the meteorological conditions.  Measured background PFT levels will be compared with those observed at other locations in the US and at other sites around the globe.

The results of the first field program will be used to refine the design of the second program, to expand the scope or focus on interesting findings that require further resolution. The PFT tests will be coordinated with the other researchers at the Super Carbon Flux site to optimize the utility of all resources. 

 

 

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Last Modified: November 12, 2009
Please forward all questions about this site to: Linda Satalino