February 24, 2000

FACT SHEET: GROUNDWATER INVESTIGATION NEAR FORMER E-20 CATCHER

Brookhaven National Laboratory (BNL), Upton NY

Contacts: DOE: Scott Mallette, 631-344-5345; BNL: Bet Zimmerman, 631-344-4225

Summary

BNL’s enhanced groundwater monitoring program has detected a narrow plume of tritium and sodium-22 at levels of approximately two times the drinking water standard. The source of the tritium and sodium-22 has been identified as activated soil used as shielding near the former E-20 Catcher located in the Alternating Gradient Synchrotron facility. BNL is taking corrective measures to prevent further releases of tritium and sodium-22, and will be conducting additional characterization studies. BNL will closely monitor the effectiveness of these actions. No tritium has been detected in potable water supply wells.

Background

bulletBNL's Environmental Management System includes a comprehensive groundwater protection program that relies heavily on pollution prevention--using operational and engineered controls to prevent contamination from entering the groundwater. Since a sole source aquifer is beneath our facility, is it a priority for BNL to protect that resource.
bulletA supporting element of the groundwater protection program is the monitoring program, used to determine whether or not the controls are effective and whether there are other problems that need to be addressed. There are over 700 monitoring wells onsite -- most of which are associated with Environmental Restoration program, and others that monitor water quality at boundaries and near potable drinking water supplies.
bulletAs part of the Groundwater Monitoring Improvements Project, more than 80 additional wells have been recently installed around active research and support operations across the Laboratory. We expect that some of these wells may detect problems in these operational areas, and will use the monitoring data to help determine what corrective actions may be needed, and whether the corrective actions are effective.

E-20 Catcher

The Collider-Accelerator (C-A) Complex is comprised of a series of particle accelerators (rings), particle injectors and several experimental halls. The Alternating Gradient Synchrotron (AGS) Ring, one of the accelerators, is about 800 meters in circumference and is divided into 12 equal segments called super-periods. The E-20 beam catcher was located at the E super-period (approximately the 5 o’clock position), and was used to capture protons that move out of acceptable pathways as they accelerate around the AGS. Like other beam loss areas within the Collider-Accelerator complex, the soil used as shielding at the E-20 Catcher is likely to have become activated by interaction with secondary particles. Rainwater permeating these soils has the potential to leach activation products (primarily sodium-22 and tritium) into groundwater.

The E-20 operated from 1984 – 1999. In 1999, a new catcher was installed at location J-10 in the J super-period. Improvements in the design of this new catcher include a poured concrete roof and a soil-crete cover. These design improvements will reduce the potential for rainwater infiltration of activated soils.

Groundwater Data

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The predominant groundwater flow direction in the E-20 catcher area is to the south-southeast. The depth to groundwater is approximately 28 to 30 feet below land surface, and the area is underlain by predominantly fine to coarse-grained sand and fine gravel.

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In December 1997, four Geoprobe wells were installed approximately 500 feet south-southeast (downgradient) of the E-20 area as part of an effort to evaluate general groundwater quality in the AGS area (conducted by the Environmental Restoration Program’s Preliminary Assessment/Site Investigation Project). Groundwater samples collected from one of these wells contained very low concentrations of tritium (approximately 560 pCi/L; or 3% of the drinking water standard of 20,000 pCi/L) and sodium-22 (24 pCi/L; or approximately 6% of the drinking water standard of 400 pCi/L). Both tritium and sodium-22 were non-detectable in samples from the other wells.

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As part of the Brookhaven National Laboratory’s Groundwater Monitoring Improvements Plan, (available online at http://www.bnl.gov/esd/gw.htm), a series of new groundwater monitoring wells were installed near a number of C-A Department beam stop, collimator and target areas, where soil activation was known or expected to occur. In early 1999, two permanent monitoring wells (064-055 and 064-056) were installed approximately 100 feet south-southeast of the E-20 catcher to better monitor groundwater quality in this region. These wells are spaced approximately 60 feet apart and abut the northwest side of Building 911 (Figure 1).

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Monitoring conducted since May 1999 showed that concentrations of tritium varied from non-detect to 5,800 pCi/L in one of the wells (064-056). Sodium-22 was detected in both wells at concentrations up to 70 pCi/L. Table 1 summarizes the calendar year 1999 monitoring data from permanent Wells 064-055 and 064-056.

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Because Well 064-056 might have been located on the edge of a more concentrated plume, BNL decided to install four additional temporary wells to further define the extent of tritium and sodium-22 in this area.

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Four Geoprobe wells were installed in January 2000. Detectable levels of tritium and sodium-22 were found in samples from three of the four temporary wells (Figure 1). The well installed furthest to the northeast (064-063) did not contain tritium or sodium above detectable levels. The highest concentrations of sodium-22 and tritium were found in well 064-065 at concentrations of 704 pCi/L and 40,400 pCi/L, respectively. These wells are located approximately 12’ and 24’ southwest of permanent well 064-056 respectively. Table 1 summarizes the results for the four Geoprobe wells.

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At a distance of approximately 100 feet downgradient of the E-20 catcher, the zone of elevated tritium and sodium-22 is estimated to be approximately 20 to 30 feet wide and situated within 10 feet of the water table (approximately 30 to 40 feet below land surface).

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As with the other beam stop areas, the E-20 is not within the immediate capture zone of any drinking water supply well, so public health is not impacted.

Corrective Actions

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In accordance with BNL's draft Groundwater Contingency Plan, regulators and the public were notified of our findings and planned corrective actions.

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BNL is in the process of installing a new cap over the E-20 catcher area to prevent further leaching of activation products. This technology has proven very successful in other areas onsite.

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BNL will install additional temporary wells to better define the downgradient extent of the plume, and may install additional permanent wells for long-term monitoring.

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Evaluation of any other actions required continues.

Other Areas within the C-A Department Complex

The Laboratory has identified 22 primary areas within the C-A Complex that catch or stop protons, with 8 target areas proximate to 8 proton stops. There are four more beam-beam interaction points at RHIC, but soil activation is expected at the non-detectable level. Secondary particles created in these areas have the potential to generate tritium and sodium-22 in adjacent soil used as shielding. Recent groundwater investigations have shown that elevated concentrations of both tritium and sodium-22 exist in groundwater in some of these areas (i.e., BLIP, g-2 and the E-20). Monitoring of other indoor beam-loss areas such as targets and collimators in the experimental halls has shown no significant impacts to groundwater quality. New facilities like RHIC and the Booster Applications Facility are have been proactively designed to prevent impacts.

Conclusions

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The enhanced groundwater monitoring network as designed enabled us to quickly characterize the area of contamination.

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BNL has taken immediate and comprehensive corrective actions to address the identified source.

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The narrow plume is not currently threatening any existing potable water supply wells— NO tritium has been detected in the closest potable water supply well, which is located to the east of E-20. BNL continues to monitor the potable water monthly as part of its routine monitoring program. The contamination is located at the center of the site and the plume is not expected to move offsite.

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The groundwater monitoring network is working as intended--the data indicated that our controls need to be enhanced, and we are taking the corrective actions listed above.

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This detection resulted from BNL’s systematic and comprehensive approach to evaluating facilities. The Laboratory is implementing this part of the Environmental Management System to collect information on groundwater quality. BNL will use the information to determine what additional actions are needed, and to continue to improve our groundwater protection program. However, groundwater monitoring is only a secondary means of protecting groundwater quality. BNL must continue to work hard to control or eliminate pollution at the source to protect groundwater quality.

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The groundwater monitoring improvements initiative will continue to assess groundwater at facilities with the potential to impact the environment. Information gathered during these activities provides input for the long-term strategy to manage sites of potential contamination and protect Long Island's drinking water supply.

Figure 1: E-20 catcher and the locations of the Geoprobe wells and permanent monitoring wells

 

Table 1
Brookhaven National Laboratory
E-20 Catcher Groundwater Investigation
January 2000
Geoprobe Well Sample Depth (BLS) Tritium (pCi/L) Reanalysis Na-22 (pCi/L)
064-063 43’-47’ <296   ND
  39’-43’ <296   ND
  35’-39’ <296   ND
  31’-35’ <296   ND
  27’-31’ NS   NS
064-064 43’-47’ 321 +/- 191   ND
  39’-43’ <296   2.5 +/- 1.3
  35’-39’ <316   102 +/- 11
  31’-35’ 5,520 +/- 377   297 +/- 35
  28’-32’ 679 +/- 219   111 +/- 13
064-065 43’-47’ <316   5.9 +/- 1.8
  39’-43’ 547 +/- 214   7.5 +/- 1.7
  35’-39’ 40,400 +/- 921 43,000 +/- 1,080 517 +/- 55
  31’-35’ 17,500 +/- 627 18,400 +/- 723 701 +/- 83
  31’-35’ (Duplicate) 15,700 +/- 590   704 +/- 78
  27’-31’ 6,600 +/- 409   543 +/- 59
064-066 43’-47’ <316   ND
  39’-43’ <316   ND
  35’-39’ <316   4.5 +/- 1.2
  31’-35’ 768 +/- 226   77.4 +/- 8.8
  28’-31’ 2,180 +/- 284   337 +/- 40
         
Permanent Monitoring Well Data Date      
064-055 May 1999 333 +/- 206   6.9
  July 1999 513 +/- 207   2.4
  Oct. 1999 656 +/- 220   ND
  Jan. 2000 Not available yet    
         
064-056 May 1999 5,800 +/- 396   219 +/-
  July 1999 <323   66 +/-
  Oct. 1999 3,840 +/- 347   70 +/-
  Jan. 2000 Not available yet    
         
Drinking Water Standard   20,000   400

ND = Not Detected R = Reanalysis NS = Not sampled BLS = Below Land Surface

Note: "<" symbols preceding a value (e.g., <304) indicates that the measured tritium value was less than the stated Minimum Detection Limit.