Condensed-Matter Physics & Materials Science Seminar

"Spin fluctuations in 122 transition metal arsenides measured using inelastic neutron scattering technique"

Presented by Aashish Sapkota, Ames Laboratory

Thursday, December 21, 2017, 1:30 pm — ISB Bldg. 734 Conf. Rm. 201 (upstairs)

122 transition metal compounds with ThCr2Si2-type structure have been extensively studied because of their wide range of interesting physical properties like superconductivity, valence fluctuations, various magnetic ground states, etc. A subset (ATM2Pn2) of this class consisting of alkaline earth metals (A), 3d transition metals (TM) and pnictogen (Pn) attracted significant interest after discovery of an unconventional superconductivity in 122 iron arsenide compounds. In 122 iron arsenide superconductors, magnetism is in close proximity to the superconductivity and the spin fluctuations are considered as a key component for the pairing mechanism for superconductivity. These properties as well as the wide range of magnetic ground states, found in ATM2As2, motivated a detail studies of the magnetism in these compounds and neutron scattering technique has been extensively used for the study. In this seminar, I will discuss our results of inelastic neutron scattering measurements of the spin fluctuations in two compounds [CaCo1.86As2 and Ca(Fe1-xCox)2As2] of ATM2Pn2 class. First, I will discuss extremely extended spin fluctuations along two directions of reciprocal space in CaCo1.86As2, which shows A-type antiferromagnetic ground states. The result suggests that CaCo1.86As2 is highly-frustrated and is a unique example of highly-frustrated square-lattice system. Next, I will discuss the evolution of the spin fluctuations in Co-doped CaFe2As2 and compare it to that of Co-doped BaFe2As2. In this part, I will also discuss a peculiar suppression of the spin fluctuations with temperature observed in Ca(Fe1-xCox)2As2, x = 0.030 compound, which shows superconducting ground state.

Hosted by: John Tranquada

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